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Sakamura, Yoshiharu*; Inoue, Tadashi*; Iwai, Takashi; Moriyama, Hirotake*
Journal of Nuclear Materials, 340(1), p.39 - 51, 2005/04
Times Cited Count:41 Percentile:91.71(Materials Science, Multidisciplinary)A new chlorination method using ZrCl in a molten salt has been investigated for the pyrometallurgical reprocessing of spent oxide fuels. UO, PuO and rare earth oxides(LaO, CeO, NdO and YO) were allowed to react with ZrCl in a LiCl-KCl eutectic salt at 500C to give a metal chloride solution and a precipitate of ZrO. By keeping the system quite still, the solution settled so that the ZrO precipitate could be separated.